Ostwald Ripening of Clusters during Protein Crystallization

Ostwald ripening, chiral crystallization, and the common-ancestor effect.

We introduce an agent-based model for advection-mediated chiral autocatalysis in which we take into account dissolution-crystallization processes through Ostwald ripening. We demonstrate that the latter phenomenon is the key to explaining previously puzzling experimental results whereby complete chiral symmetry breaking is attained from an initially unbiased mixture of seed crystals. We show th...

Kinetically suppressed ostwald ripening of Ge/Si(100) hut clusters.

Low area density Ge/Si(100) hut cluster ensembles are stable during days-long growth temperature anneals. Real-time scanning tunneling microscopy shows that all islands grow slowly at a decreasing rate throughout the anneal. Island growth depletes the Ge supersaturation that, in turn, reduces the island growth rate. A mean-field facet nucleation and growth model quantitatively predicts the obse...

Ostwald ripening pdf

Homoepitaxial Ostwald ripening

This paper reports level set simulations of the Ostwald ripening of two-dimensional homoepitaxial islands. The simulation accurately accounts for both adatom diffusion between the islands and adatom attachment/detachment processes at the island edges. We compute the time evolution of the average island size and the full island size distribution function. The results provide support for a previo...

Part I: Ostwald ripening theories

The physical basis behind the Ostwald ripening process for two-phase mixture has been reviewed in detail, using the various theories developed to describe this process. The Ostwald ripening, also termed second phase coarsening, is generally thought to be slow, diffusion-controlled process which occurs subsequent to phase separation under extremely small under-saturation levels. The major advanc...